Characteristics of atmospheric transport into the Antarctic troposphere

We have developed a 5.5 year climatology of atmospheric transport into the Antarctic troposphere, which uses the same data set and methods as described in a recent study for the Arctic. This allows direct comparisons of transport properties for the two polar regions. The climatology is based on a simulation with the Lagrangian particle dispersion model FLEXPART, where the model atmosphere was globally filled with particles. Transport characteristics as well as emission sensitivities were derived from 6 hourly particle positions. We found that the probability for near-surface air to originate from the stratosphere on a time scale of 10 days is an order of magnitude higher near the South Pole than near the North Pole, a result of higher topography and descent that partly compensates for the flow of air down the Antarctic Plateau with the katabatic winds. The stratospheric influence is largest in fall, which is opposite to the seasonality in the Arctic. Stratospheric influence is much smaller over the shelf ice regions and in a band around Antarctica. The average time for which air near the surface has been exposed to continuous darkness in July (continuous light in January) is longest over the Ronne Ice Shelf and Ross Ice Shelf at ∼11 days (20 days). We calculated how sensitive Antarctic air masses are to emission input up to 30 days before arriving in Antarctica if removal processes are ignored. The emission sensitivity shows strong meridional gradients and, as a result, is generally low over South America, Africa, and Australia. For a 10 day time scale, the largest emission sensitivities over these continents are 1–2 orders of magnitude smaller than over Eurasia for transport to the Arctic, showing that foreign continents have a much smaller potential to pollute the Antarctic than the Arctic troposphere. Emission sensitivities and derived black carbon (BC) source contributions over South America, Africa, and Australia are substantially (a factor 10 for Africa) larger in winter than in summer. In winter, biomass burning contributes more BC than anthropogenic sources. For typical aerosol lifetimes of 5–10 days, ship emissions south of 60°S account for half of the total BC concentrations in the lowest 1000 m of the atmosphere south of 70°S in December. The increasing number of tourists visiting Antarctica and fishing vessels operating close to Antarctica are, therefore, a matter of concern.