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Using a ground-based microwave radiometer at Troll Station, Antarctica (72°S, 2.5°E,L = 4.76), we have observed a decrease of 20–70% in the mesospheric ozone, coincident with increased nitric oxide, between 60 km and 75 km altitude associated with energetic electron precipitation (E > 30 keV) during a moderate geomagnetic storm (minimum Dst of −79 nT) in late July 2009. NOAA satellite data were used to identify the precipitating particles and to characterize their energy, spatial distribution and temporal variation over Antarctica during this isolated storm. Both the ozone decrease and nitric oxide increase initiate with the onset of the storm, and persist for several days after the precipitation ends, descending in the downward flow of the polar vortex. These combined data present a unique case study of the temporal and spatial morphology of chemical changes induced by electron precipitation during moderate geomagnetic storms, indicating that these commonplace events can cause significant effects on the middle mesospheric ozone distribution.

Radar power returned from the basal interface along a 42 km long profile over an ice-rise promontory and the adjacent Roi Baudouin ice shelf, Dronning Maud Land, East Antarctica, is analyzed to infer spatial variations in basal reflectivity and hence the basal environment. Extracting basal reflectivity from basal returned power requires an englacial attenuation model. We estimate attenuation in two ways: (1) using a temperature-dependent model with input from thermomechanical ice-flow models; and (2) using a radar method that linearly approximates the geometrically corrected returned power with ice thickness. The two methods give different results. We argue that attenuation calculated using a modeled temperature profile is more robust than the widely used radar method, especially in locations where depth-averaged attenuation varies spatially or where the patterns of basal reflectivity correlate with the patterns of the ice thickness.

Long term atmospheric mercury measurements in the Southern Hemisphere are scarce and in Antarctica completely absent. Recent studies have shown that the Antarctic continent plays an important role in the global mercury cycle. Therefore, long term measurements of gaseous elemental mercury (GEM) were initiated at the Norwegian Antarctic Research Station, Troll (TRS) in order to improve our understanding of atmospheric transport, transformation and removal processes of GEM. GEM measurements started in February 2007 and are still ongoing, and this paper presents results from the first four years. The mean annual GEM concentration of 0.93 ± 0.19 ng m−3 is in good agreement with other recent southern-hemispheric measurements. Measurements of GEM were combined with the output of the Lagrangian particle dispersion model FLEXPART, for a statistical analysis of GEM source and sink regions. It was found that the ocean is a source of GEM to TRS year round, especially in summer and fall. On time scales of up to 20 days, there is little direct transport of GEM to TRS from Southern Hemisphere continents, but sources there are important for determining the overall GEM load in the Southern Hemisphere and for the mean GEM concentration at TRS. Further, the sea ice and marginal ice zones are GEM sinks in spring as also seen in the Arctic, but the Antarctic oceanic sink seems weaker. Contrary to the Arctic, a strong summer time GEM sink was found, when air originates from the Antarctic plateau, which shows that the summertime removal mechanism of GEM is completely different and is caused by other chemical processes than the springtime atmospheric mercury depletion events. The results were corroborated by an analysis of ozone source and sink regions.

The mass balance of Antarctica is one of the crucial factors for determining sea-level change in a warming climate. The marginal zones of the continent, namely the ice shelves, are most sensitive to climate change. During the 2009/10 austral summer an extensive glaciological field campaign was carried out on Fimbulisen, an ice shelf in East Antarctica, to investigate its recent surface mass balance. Shallow (10–18 m) firn cores were drilled and accumulation rates and stable-isotope ratios determined. For firn-core dating, two different methods were compared: (1) seasonal variations of stable oxygen isotope ratios (δ18O), and (2) dielectric profiling, including using the volcanic eruptions of Pinatubo, Philippines (1991), and El Chichόn, Mexico (1982), as time markers. The mean annual accumulation for the period 1992–2009 ranges from 298 to 349 mmw.e. a–1. The interannual variability at the drilling sites is >30%. Accumulation rates show a weak decreasing trend during the past 20–30 years, which is statistically significant only for one of the cores. Stable-isotope ratios were compared to the snowfall temperature of Neumayer station. Neither the temperatures nor the δ18O values show any trend for the investigated time period.

We compare the present and last interglacial periods as recorded in Antarctic water stable isotope records now available at various temporal resolutions from six East Antarctic ice cores: Vostok, Taylor Dome, EPICA Dome C (EDC), EPICA Dronning Maud Land (EDML), Dome Fuji and the recent TALDICE ice core from Talos Dome. We first review the different modern site characteristics in terms of ice flow, meteorological conditions, precipitation intermittency and moisture origin, as depicted by meteorological data, atmospheric reanalyses and Lagrangian moisture source diagnostics. These different factors can indeed alter the relationships between temperature and water stable isotopes. Using five records with sufficient resolution on the EDC3 age scale, common features are quantified through principal component analyses. Consistent with instrumental records and atmospheric model results, the ice core data depict rather coherent and homogenous patterns in East Antarctica during the last two interglacials. Across the East Antarctic plateau, regional differences, with respect to the common East Antarctic signal, appear to have similar patterns during the current and last interglacials. We identify two abrupt shifts in isotopic records during the glacial inception at TALDICE and EDML, likely caused by regional sea ice expansion. These regional differences are discussed in terms of moisture origin and in terms of past changes in local elevation histories, which are compared to ice sheet model results. Our results suggest that elevation changes may contribute significantly to inter-site differences. These elevation changes may be underestimated by current ice sheet models.

We report the first ground-based passive microwave observations made from Troll station, Antarctica, which show enhanced mesospheric nitric oxide (NO) volume mixing ratio reaching levels of 1.2 ppmv, or 2–3 orders of magnitude above background, at 70–80 km during small, relatively isolated geomagnetic storms in 2008. The mesospheric NO peaked 2 days after enhanced NO at higher altitudes (110–150 km) measured by the SABER satellite, and 2 days after peaks in the >30 keV and >300 keV electron flux measured by POES, although the 300 keV electron flux remained high. High time resolution data shows that mesospheric NO was enhanced at night and decayed during the day and built up to high levels over a period of 3–4 days. The altitude profile of mesospheric NO suggests direct production by ∼300 keV electron precipitation. Simulations using the Sodankylä Ion and Neutral Chemistry model show that the delay between thermospheric and mesospheric NO enhancements was primarily a result of the weaker production rate at lower altitudes by ∼300 keV electrons competing against strong day-time losses.

We report on ground-based atmospheric measurements and emission estimates of the four anthropogenic hydrofluorocarbons (HFCs) HFC-365mfc (CH3CF2CH2CF3, 1,1,1,3,3-pentafluorobutane), HFC-245fa (CHF2CH2CF3, 1,1,1,3,3-pentafluoropropane), HFC-227ea (CF3CHFCF3, 1,1,1,2,3,3,3-heptafluoropropane), and HFC-236fa (CF3CH2CF3, 1,1,1,3,3,3-hexafluoropropane). In situ measurements are from the global monitoring sites of the Advanced Global Atmospheric Gases Experiment (AGAGE), the System for Observations of Halogenated Greenhouse Gases in Europe (SOGE), and Gosan (South Korea). We include the first halocarbon flask sample measurements from the Antarctic research stations King Sejong and Troll. We also present measurements of archived air samples from both hemispheres back to the 1970s. We use a two-dimensional atmospheric transport model to simulate global atmospheric abundances and to estimate global emissions. HFC-365mfc and HFC-245fa first appeared in the atmosphere only ∼1 decade ago; they have grown rapidly to globally averaged dry air mole fractions of 0.53 ppt (in parts per trillion, 10−12) and 1.1 ppt, respectively, by the end of 2010. In contrast, HFC-227ea first appeared in the global atmosphere in the 1980s and has since grown to ∼0.58 ppt. We report the first measurements of HFC-236fa in the atmosphere. This long-lived compound was present in the atmosphere at only 0.074 ppt in 2010. All four substances exhibit yearly growth rates of >8% yr−1 at the end of 2010. We find rapidly increasing emissions for the foam-blowing compounds HFC-365mfc and HFC-245fa starting in ∼2002. After peaking in 2006 (HFC-365mfc: 3.2 kt yr−1, HFC-245fa: 6.5 kt yr−1), emissions began to decline. Our results for these two compounds suggest that recent estimates from long-term projections (to the late 21st century) have strongly overestimated emissions for the early years of the projections (∼2005–2010). Global HFC-227ea and HFC-236fa emissions have grown to average values of 2.4 kt yr−1 and 0.18 kt yr−1 over the 2008–2010 period, respectively.

Holocene climate variability in the southeast Atlantic sector of the Southern Ocean and Antarctic is assessed and quantified through integration of available marine sediment core and Antarctic ice core data. We use summer sea surface temperature (SSST) and sea ice presence (SIP) reconstructions from two marine sediment cores recovered north (50 °S) and south (53.2 °S) of the present day Antarctic Polar Front (APF), as well as an atmospheric temperature and sea ice proxy from the EPICA ice core from Dronning Maud Land (EDML). We find reasonably good agreement in the timing of climate evolution in the analyzed series. Almost all records show a gradual glacial-to-Holocene climate transition, interrupted by the Antarctic cold reversal around 13 000 cal yr BP, and early Holocene climatic optimum (HCO) at about 11 000 cal yr BP. During the early HCO, the seasonal ice cover retreats to south of 53 °S; it then readvances in the course of the mid- to late Holocene. The maximum winter sea ice edge position during the recent 10 000 years varied mainly within 51–53 °S, with sporadic growth to north of 50 °S, a position similar to that during the last glacial. The onset of the Neoglacial period after ca 4000 yr BP is associated with a steepening of the SSST gradient between the marine core sites, strengthening of the westerlies and cooling in the inland ice sheet. The agreement in timing between elevated SSST during the early HCO and decreased deuterium excess in EDML and other ice cores from different locations in the East Antarctic suggests that the retreat of sea ice during the early HCO and weakening of the APF was a general feature of the East Antarctic climate during that time.

Snow accumulation and its variability on the East Antarctic plateau are poorly understood due to sparse and regionally confined measurements. We present a 5.3 GHz (C-band) ground-penetrating radar (GPR) profile with a total length of 860 km recovered during the joint Norwegian–US International Polar Year traverse 2007/08. Mean surface mass balance (SMB) over the last 200 years was derived from the GPR data by identifying the volcanic deposition of the Tambora eruption in 1815. It varies between 9.1 and 37.7 kg m−2 a−1 over the profile, with a mean of 23.7 kg m−2 a−1 and a standard deviation of 4.7 kg m−2 a−1. The 200 year SMB estimated is significantly lower than most of the SMB estimates over shorter time periods in this region. This can be partly explained by a SMB minimum in the vicinity of the ice divide. However, it is more likely that a recent increase in SMB observed by several studies is largely responsible for the observed discrepancy.

An extreme precipitation event that influenced almost the whole polar plateau of Dronning Maud Land, Antarctica, is investigated using Antarctic Mesoscale Prediction System archive data. For the first time a high-resolution atmospheric model especially adapted for polar regions was used for such a study in Dronning Maud Land. The outstanding event of 21–25 February 2003 was connected to a strong north-westerly flow, caused by a blocking high above eastern Dronning Maud Land, that persisted for several days and brought unusually large levels of moisture to the Antarctic Plateau. This weather situation is most effective in bringing precipitation to high-altitude interior Antarctic ice-core drilling sites, where precipitation in the form of diamond dust usually dominates. However, a few such precipitation events per year can account for a large percentage of the annual accumulation, which can cause a strong bias in ice-core data. Additionally, increased temperatures and wind speeds during these events need to be taken into account for the correct climatic interpretation of ice cores. A better understanding of the frequency of occurrence of intermittent precipitation in the interior of Antarctica in past and future climates is necessary for both palaeoclimatological studies and estimates of future sea-level change.

[1] Ground-based accumulation measurements are scarce on the high East Antarctic plateau, but highly necessary for model validation and the interpretation of satellite data for the determination of Antarctic mass balance. Here, we present accumulation results obtained from four shallow firn cores drilled in the Antarctic summer season 2007/2008. The cores were drilled along the first leg of the Norwegian-US IPY traverse through East Antarctica, visiting sites like Plateau Station and Pole of Relative Inaccessibility that have been covered by the South Pole Queen Maud Land Traverses (SPQMLT) in the 1960s. Accumulation has been determined from volcanic chronology established from the conductivity records measured by dielectric profiling (DEP). The Tambora 1815/unknown 1809 double peak is clearly visible in the conductivity data and serves as a reliable time marker. Accumulation rates averaged over the period 1815–2007 are in the range of 16 to 32 kg m−2 a−1, somewhat lower than expected from the SPQMLT data. The spatial pattern is mainly influenced by elevation and continentality. Three of the firn cores show a decrease of more than 20% in accumulation for the time period 1815–2007 in relation to accumulation rates during the period 1641–1815. The spatial representativity of the firn cores is assessed by ground-penetrating radar, showing a rather smoothly layered pattern around the drill sites. Validation of the DEP results is utilized by comparison with chemistry data, proving the validity of the DEP method for dating firn cores. The results help understanding the status of the East Antarctic ice sheet and will be important for e.g. future model-derived estimates of the mass balance of Antarctica.