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The atmospheric observatory at the Norwegian Research Station Troll in Queen Maud Land, Antarctica, holds, since February 2007, the first all-year Antarctic atmospheric aerosol particle number size distribution measurements. These are colocated with measurements of the aerosol absorption and spectral scattering coefficients. In June 2007, this instrument set observed an aerosol whose properties were indicative of a biomass burning aerosol. These properties included two log-normal size distribution modes with median particle diameters of 0.105 μm and 0.36 μm, sharply falling off to smaller and larger sizes, and peaks in scattering and absorption coefficient. With backward plume calculations of the Lagrangian transport model FLEXPART and the MODIS fire activity product, a source-receptor relationship was established between biomass burning events in Central Brazil and the aerosol seen at Troll. This is the first direct evidence that the Antarctic continent is susceptible to emissions from as far north as Southern tropical latitudes.

The Troll Atmospheric Station in Antarctica (72°01'S, 2°32'E, 1309 m a.s.l.) was established and put into operation in early 2007. The main foci of the measurement programme are pollution and aerosols in the transition zone between the coastal zone and the inland ice plateau, complementing existing observation programmes along the Antarctic coast and on the Antarctic Plateau. After one year of operation, the monitoring programme is fully operative, and a comprehensive set of data is being analysed. As far as comparable data are available, there is satisfactory agreement between previous and new data. Both aerosol data and measurements of pollution indicate the episodic influence of coastal air masses throughout the year. Background values of medium long-lived pollutants such as CO, O3 and Hg are up to 50% lower than at corresponding Arctic sites (depending on the season), but are still significant. Total ozone and UV doses manifest the recurring Antarctic stratospheric ozone hole, which was moderately severe, but very persistent in 2007. Specific episodes of elevated aerosol concentration and mercury activation are currently under detailed investigation, and will be published separately.

Observations of snow properties, superimposed ice, and atmospheric heat fluxes have been performed on first-year and second-year sea ice in the western Weddell Sea, Antarctica. Snow in this region is particular as it does usually survive summer ablation. Measurements were performed during Ice Station Polarstern (ISPOL), a 5-week drift station of the German icebreaker RV Polarstern. Net heat flux to the snowpack was 8 W m−2, causing only 0.1 to 0.2 m of thinning of both snow cover types, thinner first-year and thicker second-year snow. Snow thinning was dominated by compaction and evaporation, whereas melt was of minor importance and occurred only internally at or close to the surface. Characteristic differences between snow on first-year and second-year ice were found in snow thickness, temperature, and stratigraphy. Snow on second-year ice was thicker, colder, denser, and more layered than on first-year ice. Metamorphism and ablation, and thus mass balance, were similar between both regimes, because they depend more on surface heat fluxes and less on underground properties. Ice freeboard was mostly negative, but flooding occurred mainly on first-year ice. Snow and ice interface temperature did not reach the melting point during the observation period. Nevertheless, formation of discontinuous superimposed ice was observed. Color tracer experiments suggest considerable meltwater percolation within the snow, despite below-melting temperatures of lower layers. Strong meridional gradients of snow and sea-ice properties were found in this region. They suggest similar gradients in atmospheric and oceanographic conditions and implicate their importance for melt processes and the location of the summer ice edge.

The seasonality of moisture sources for precipitation in Antarctica is studied with a Lagrangian moisture source diagnostic. Moisture origin for precipitation in Antarctica has strongly asymmetric properties, which are related to the Antarctic topography, seasonal sea ice coverage, and the land/ocean contrasts in the mid-latitudes of the southern hemisphere. The highest altitudes of the East Antarctic ice shield, where major ice cores have been drilled, have mean source latitudes of 45–40°S year-round. This finding contrasts to results from previous Lagrangian studies which detected a more southerly moisture origin due to too short trajectories. Now, results from Lagrangian moisture source diagnostics are consistent with findings from general circulation models with tagged tracers. Thus, both approaches can serve as a common benchmark for the interpretation of moisture source indicators based on stable isotopes, such as deuterium excess, in Antarctic ice cores.

The acquisition and interpretation of increasingly high-resolution climate data from polar ice and firn cores motivates the question: What is the finest depth or timescale on which measurements on cores arrayed over a given area correlate? We analyze dated depth series of electrical and oxygen isotope measurements from a spatial array of firn cores with 3.5–7 km spacing in Dronning Maud Land, Antarctica, each with a temporal span of approximately 200 years. We use wavelet analysis to decompose the series into components associated with changes of averages on different scales, and thus deduce which scales are dominated by environmental noise, and which may contain a common signal. We find that common signals in electrical records have timescales of approximately 1–3 years. We identify only one electrical signal which rises significantly above the background in our 200-year records, evidently corresponding to the Tambora eruption. Several smaller signals correlate in a few of pairs of cores, one of which may correspond to a known volcanic event, but the others appear to be spurious. We present a simulation-based method for testing the significance of apparent electrical signal correlations, and highlight the importance of accurate relative dating between cores. In the case of oxygen-isotope records, we find, surprisingly, no significant correlation on any scale in the records, for any of the pairs of cores. There is, however, a weak trend toward positive correlation at longer timescales (up to 16 years). Statistical theory for the relevant confidence intervals and the observed statistics of the records permit estimation of the length of a data series necessary to reliably detect a hypothetical correlation equal to that observed. For the highest correlation observed on 16-year scales, core records of about 380 years (approximately 30 m at the Dronning Maud Land site) would be necessary to establish significance.

An evaluation is made of ozone profiles retrieved from measurements of the nadir-viewing Global Ozone Monitoring Experiment (GOME) instrument. Currently, four different approaches are used to retrieve ozone profile information from GOME measurements, which differ in the use of external information and a priori constraints. In total nine different algorithms will be evaluated exploiting the optimal estimation (Royal Netherlands Meteorological Institute, Rutherford Appleton Laboratory, University of Bremen, National Oceanic and Atmospheric Administration, Smithsonian Astrophysical Observatory), Phillips-Tikhonov regularization (Space Research Organization Netherlands), neural network (Center for Solar Energy and Hydrogen Research, Tor Vergata University), and data assimilation (German Aerospace Center) approaches. Analysis tools are used to interpret data sets that provide averaging kernels. In the interpretation of these data, the focus is on the vertical resolution, the indicative altitude of the retrieved value, and the fraction of a priori information. The evaluation is completed with a comparison of the results to lidar data from the Network for Detection of Stratospheric Change stations in Andoya (Norway), Observatoire Haute Provence (France), Mauna Loa (Hawaii), Lauder (New Zealand), and Dumont d'Urville (Antarctic) for the years 1997–1999. In total, the comparison involves nearly 1000 ozone profiles and allows the analysis of GOME data measured in different global regions and hence observational circumstances. The main conclusion of this paper is that unambiguous information on the ozone profile can at best be retrieved in the altitude range 15–48 km with a vertical resolution of 10 to 15 km, precision of 5–10%, and a bias up to 5% or 20% depending on the success of recalibration of the input spectra. The sensitivity of retrievals to ozone at lower altitudes varies from scheme to scheme and includes significant influence from a priori assumptions.

A solar occultation sensor, the Improved Limb Atmospheric Spectrometer (ILAS)-II, measured 5890 vertical profiles of ozone concentrations in the stratosphere and lower mesosphere and of other species from January to October 2003. The measurement latitude coverage was 54–71°N and 64–88°S, which is similar to the coverage of ILAS (November 1996 to June 1997). One purpose of the ILAS-II measurements was to continue such high-latitude measurements of ozone and its related chemical species in order to help accurately determine their trends. The present paper assesses the quality of ozone data in the version 1.4 retrieval algorithm, through comparisons with results obtained from comprehensive ozonesonde measurements and four satellite-borne solar occultation sensors. In the Northern Hemisphere (NH), the ILAS-II ozone data agree with the other data within ±10% (in terms of the absolute difference divided by its mean value) at altitudes between 11 and 40 km, with the median coincident ILAS-II profiles being systematically up to 10% higher below 20 km and up to 10% lower between 21 and 40 km after screening possible suspicious retrievals. Above 41 km, the negative bias between the NH ILAS-II ozone data and the other data increases with increasing altitude and reaches 30% at 61–65 km. In the Southern Hemisphere, the ILAS-II ozone data agree with the other data within ±10% in the altitude range of 11–60 km, with the median coincident profiles being on average up to 10% higher below 20 km and up to 10% lower above 20 km. Considering the accuracy of the other data used for this comparative study, the version 1.4 ozone data are suitably used for quantitative analyses in the high-latitude stratosphere in both the Northern and Southern Hemisphere and in the lower mesosphere in the Southern Hemisphere.

Measuring ultraviolet radiation in the Antarctic region, where weather conditions are extremely challenging, is a demanding task. Proper quality control of the measurements and quality assurance of the data, which are the basis of all scientific use of data, has to be especially well planned and executed. In this paper we show the importance of proper quality assurance and describe the methods used to successfully operate the NILU-UV multichannel radiometers of the Antarctic network stations at Ushuaia, 54°S, and Marambio, 64°S. According to our experience, even though multichannel instruments are supposed to be rather stable as a function of time, severe drifts can occur in the sensitivity of the channels under these harsh conditions. During 2000–2003 the biggest drifts were 35%, both at Ushuaia and Marambio, with the sensitivity of the channels dropping at different rates. Without proper corrections in the data, this would have seriously affected the calculated UV dose rates. As part of the quality assurance of the network a traveling reference NILU-UV, which was found to be stable, was used to transfer the desired irradiance scale to the site NILU-UV data. Relative lamp tests were used to monitor the stability of the instruments. Each site NILU-UV was scaled channel by channel to the traveling reference by performing solar comparisons. The method of scaling each channel separately was found to be successful, even though the differences between the raw data of the site NILU-UV and the reference instruments were, before the data correction, as much as 40%. After the correction, the mean ratios of erythemally weighted UV dose rates measured during the solar comparisons in 2000–2003 between the reference NILU-UV and the site NILU-UV were 1.007 ± 0.011 and 1.012 ± 0.012 for Ushuaia and Marambio, respectively, when the solar zenith angle varied up to 80°. These results make possible the scientific use of NILU-UV data measured simultaneously at quite different locations, e.g., the Antarctic and Arctic, and the method presented is also practicable for other multichannel radiometer networks.

This paper presents modeled surface and subsurface melt fluxes across near-coastal Antarctica. Simulations were performed using a physical-based energy balance model developed in conjunction with detailed field measurements in a mixed snow and blue-ice area of Dronning Maud Land, Antarctica. The model was combined with a satellite-derived map of Antarctic snow and blue-ice areas, 10 yr (1991–2000) of Antarctic meteorological station data, and a high-resolution meteorological distribution model, to provide daily simulated melt values on a 1-km grid covering Antarctica. Model simulations showed that 11.8% and 21.6% of the Antarctic continent experienced surface and subsurface melt, respectively. In addition, the simulations produced 10-yr averaged subsurface meltwater production fluxes of 316.5 and 57.4 km3 yr−1 for snow-covered and blue-ice areas, respectively. The corresponding figures for surface melt were 46.0 and 2.0 km3 yr−1, respectively, thus demonstrating the dominant role of subsurface over surface meltwater production. In total, computed surface and subsurface meltwater production values equal 31 mm yr−1 if evenly distributed over all of Antarctica. While, at any given location, meltwater production rates were highest in blue-ice areas, total annual Antarctic meltwater production was highest for snow-covered areas due to its larger spatial extent. The simulations also showed higher interannual meltwater variations for surface melt than subsurface melt. Since most of the produced meltwater refreezes near where it was produced, the simulated melt has little effect on the Antarctic mass balance. However, the melt contribution is important for the surface energy balance and in modifying surface and near-surface snow and ice properties such as density and grain size.

The 2002 Southern Hemisphere final warming occurred early, following an unusually active winter and the first recorded major warming in the Antarctic. The breakdown of the stratospheric polar vortex in October and November 2002 is examined using new satellite observations from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument aboard the European Space Agency (ESA) Environment Satellite (ENVISA7-) and meteorological analyses, both high-resolution fields from the European Centre for Medium-Rangc Weather Forecasts and the coarser Met Office analyses. The results derived from MIPAS observations are compared to measurements and inferences from well-validated solar occultation satellite instruments [Halogen Occultation Experiment (HALOE), Polar Ozone and Aerosol Measurement lit (POAM III), and Stratospheric Aerosol and Gas Experiments II and III (SAGE II and III)] and to finescale tracer fields reconstructed by transporting trace gases based oil MIPAS or climatological data using a reverse-trajectory method. These comparisons confirm the features in the MIPAS data and the interpretation of the evolution of the flow during the vortex decay revealed by those features. Mapped ozone and water vapor from MIPAS and the analyzed isentropic potential vorticity vividly display the vortex breakdown, which occurred earlier than usual. A large tongue of vortex air was pulled out westward and coiled up in an anticyclone, while the vortex core remnant shrank and drifted eastward and equatorward over the South Atlantic. By roughly mid-November, the vortex remnant at 10 mb had shrunk below scales resolved by the satellite observations, while a vortex core remained in the lower stratosphere.

This paper presents atmospheric concentrations of ethane, propane, acetylene, and methyl chloride, inferred from firn air by using a numerical one-dimensional firn diffusion model. The firn air was collected on the Antarctic plateau in Dronning Maud Land during the Norwegian Antarctic Research Expedition (NARE) 2000/2001. The influences of seasonal variations in temperature and pressure and the variation in accumulation rate were studied and are not negligible, but appear to cancel each other out if all variability is taken into account. This paper also demonstrates that firn air from the uppermost firn layer (30 m) can be used to derive seasonal cycles of these trace gases, without needing a year-round facility. These cycles display higher atmospheric mixing ratios during the Antarctic winter and lower atmospheric mixing ratios in summer. The cycles for the year 2000 show amplitudes of 140 ± 25 ppt for ethane, 30 ± 10 ppt for propane, 24 ± 6 ppt for acetylene, and 40 ± 20 ppt for methyl chloride. For ethane and propane the amplitudes and months of maximum atmospheric concentration (phase) are in reasonable agreement with year-round measurements at the South Pole and Baring Head (New Zealand). The amplitudes for methyl chloride and acetylene are significantly greater than seen in year-round measurements at the South Pole and at Neumayer (Antarctica), although the phase is in line. While biomass burning and removal by OH radicals can partially explain these large amplitudes, the exact cause still remains unclear for methyl chloride and acetylene.

In March 2002 the European Space Agency (ESA) launched the polar-orbiting environmental satellite Envisat. One of its nine instruments is the Global Ozone Monitoring by Occultation of Stars (GOMOS) instrument, which is a medium-resolution stellar occultation spectrometer measuring vertical profiles of ozone. In the first year after launch a large group of scientists performed additional measurements and validation activities to assess the quality of Envisat observations. In this paper, we present validation results of GOMOS ozone profiles from comparisons to microwave radiometer, balloon ozonesonde, and lidar measurements worldwide. Thirty-one instruments/launch sites at twenty-five stations ranging from the Arctic to the Antarctic joined in this activity. We identified 6747 collocated observations that were performed within an 800-km radius and a maximum 20-hour time difference of a satellite observation, for the period between 1 July 2002 and 1 April 2003. The GOMOS data analyzed here have been generated with a prototype processor that corresponds to version 4.02 of the operational GOMOS processor. The GOMOS data initially contained many obviously unrealistic values, most of which were successfully removed by imposing data quality criteria. Analyzing the effect of these criteria indicated, among other things, that for some specific stars, only less than 10% of their occultations yield an acceptable profile. The total number of useful collocated observations was reduced to 2502 because of GOMOS data unavailability, the imposed data quality criteria, and lack of altitude overlap. These collocated profiles were compared, and the results were analyzed for possible dependencies on several geophysical (e.g., latitude) and GOMOS observational (e.g., star characteristics) parameters. We find that GOMOS data quality is strongly dependent on the illumination of the limb through which the star is observed. Data measured under bright limb conditions, and to a certain extent also in twilight limb, should be used with caution, as their usability is doubtful. In dark limb the GOMOS data agree very well with the correlative data, and between 14- and 64-km altitude their differences only show a small (2.5–7.5%) insignificant negative bias with a standard deviation of 11–16% (19–63 km). This conclusion was demonstrated to be independent of the star temperature and magnitude and the latitudinal region of the GOMOS observation, with the exception of a slightly larger bias in the polar regions at altitudes between 35 and 45 km.

A large database of rocket measurements of the D-region electron concentration has been studied. The data were obtained at four sites in the Antarctic (Molodezhnaya and Syowa) and Arctic (Heiss Island, and Andøya/Kiruna). The electron densities were analysed in terms of their variations with solar zenith angle, geomagnetic activity and atmospheric temperature. We found that there is a particle ionisation source in the auroral oval even in quiet conditions. The energy of the particles is such, that they penetrate down to 85km, are partially absorbed between 85 and 80km but do not penetrate (are completely absorbed) below 75km. Analysis of the dependence of the electron concentration [e] on the daily sum of Kp indices, ∑Kp, shows that at all heights considered there is an increase of [e] with ∑Kp up to some saturation value of ∑Kp and beyond this level [e] is either constant (with large scatter of the data) or even decreases. This indicates that when the auroral oval expands with increasing geomagnetic activity, a particular station may move from a position outside or at the boundary of the oval, to a position inside the polar cap. An attempt is made to find the temperature dependence of the electron concentration. It is found that [e] at 75 and 80km increases with temperature T. Analysis of the flights conducted during noctilucent cloud (NLC) events at Andøya/Kiruna reveals a strong dependence of [e] on ∑Kp at 80 and 85km. This dependence is stronger and better defined than that for the entire data set. This may be explained by the low mesopause temperatures observed in summer when NLC occur. A comparison of the electron density data sets with empirical and theoretical models is presented and during quiet magnetic conditions a good agreement with mid-latitude models is found.

This project was undertaken by the Norwegian Polar Institute for the Norwegian Petroleum Directorate (Oljedirektoratet) as support for planning of marine geophysical surveys offshore from Dronning Maud Land (DML), Antarctica. The project was carried out by scientists Olga Pavlova and Jan-Gunnar Winther at the Norwegian Polar Institute under the direction of Morten Sand at the Norwegian Petroleum Directorate. The main objectives of the project were to: a) calculate 10-day average historical (i.e., 1978-1996) sea ice concentrations off DML for the months of December through April b) identify the minimum and maximum sea ice extent occurring in the period 1978-1996 c) present the above information graphically. Daily microwave satellite data covering the period 1978-1996 with 25 x 25 km spatial resolution were used as basis for this study (see text below for description of data set).

Ground-based zenith sky UV–visible measurements of stratospheric bromine monoxide (BrO) slant column densities are compared with simulations from the SLIMCAT three-dimensional chemical transport model. The observations have been obtained from a network of 11 sites, covering high and midlatitudes of both hemispheres. This data set gives for the first time a near-global picture of the distribution of stratospheric BrO from ground-based observations and is used to test our current understanding of stratospheric bromine chemistry. In order to allow a direct comparison between observations and model calculations, a radiative transfer model has been coupled to the chemical model to calculate simulated slant column densities. The model reproduces the observations in general very well. The absolute amount of the BrO slant columns is consistent with a total stratospheric bromine loading of 20 ± 4 ppt for the period 1998–2000, in agreement with previous estimates. The seasonal and latitudinal variations of BrO are well reproduced by the model. In particular, the good agreement between the observed and modeled diurnal variation provides strong evidence that the BrO-related bromine chemistry is correctly modeled. A discrepancy between observed and modeled BrO at high latitudes during events of chlorine activation can be resolved by increasing the rate constant for the reaction BrO + ClO → BrCl + O2 to the upper limit of current recommendations. However, other possible causes of the discrepancy at high latitudes cannot be ruled out.

A large set of rocket measurements of the electron concentration [e] in the upper D region at four rocket sites (Molodezhnaya (Antarctic), Heiss Island (Arctic), Syowa (Antarctic), and Andoya/Kiruna (Arctic)) is considered. The dependence of [e] on the solar zenith angle X and geomagnetic activity index ∑Kp is analyzed. It has been shown that, the spread in [e] values reaches two orders of magnitude at any assigned value of χ. Nevertheless, it is possible to draw a lower envelope for the entire set of points and to obtain the [e] variation with χ in undisturbed conditions. In an analysis of the envelopes, it is seen that a corpuscular ionization source (presumably, electrons with an energy of above 40 keV) exists in the nonsunlit D region even in quiet conditions. An analysis of the electron concentration dependence on the daily sum of ∑Kp indices (∑Kp) shows that, at all heights considered, increases [e] with increasing ∑Kp to a certain boundary value ∑Kp and then remains either constant (with a rather wide spread in the data) or even decreases. This saturation effect may be caused by the auroral oval equatorward motion. As a result of this motion the site position may change: it may move toward the boundary between the auroral oval and polar cap or even be within the latter. The slope k of the [e] variation plotted versus ∑Kp at different χ is considered. It is shown that k grows with increasing χ and is maximal at χ> 100°.