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The metamorphic basement of the Heimefrontfjella in western Dronning Maud Land (Antarctica) forms the western margin of the major ca. 500 million year old East African/East Antarctic Orogen that resulted from the collision of East Antarctica and greater India with the African cratons. The boundary between the tectonothermally overprinted part of the orogen and its north-western foreland is marked by the subvertical Heimefront Shear Zone. North-west of the Heimefront Shear Zone, numerous low-angle dipping ductile thrust zones cut through the Mesoproterozoic basement. Petrographic studies, optical quartz c-axis analyses and x-ray texture goniometry of quartz-rich mylonites were used to reveal the conditions that prevailed during the deformation. Mineral assemblages in thrust mylonites show that they were formed under greenschist-facies conditions. Quartz microstructures are characteristic of the subgrain rotation regime and oblique quartz lattice preferred orientations are typical of simple shear-dominated deformation. In contrast, in the Heimefront Shear Zone, quartz textures indicate mainly flattening strain with a minor dextral rotational component. These quartz microstructures and lattice preferred orientations show signs of post-tectonic annealing following the tectonic exhumation. The spatial relation between the sub-vertical Heimefront Shear Zone and the low-angle thrusts can be explained as being the result of strain partitioning during transpressive deformation. The pure-shear component with a weak dextral strike-slip was accommodated by the Heimefront Shear Zone, whereas the north–north-west directed thrusts accommodate the simple shear component with a tectonic transport towards the foreland of the orogen. Keywords: Dronning Maud Land; quartz microfabrics; X-ray texture goniometry; shear zones; mylonites.

Kommersielle fiskerier kan påvirke marine økosystemer og bestander av topp-predatorer som sjøfugl. I Sørishavet foregår et ekstensivt fiske etter Antarktisk krill (Euphausia superba), og dette er antatt å øke. En sammenligning av fordeling og uttak hos fiskeriene og tilsvarende hos topp-predatorene er nødvendig for å forutsi fiskerirelaterte påvirkninger på krillavhengige predatorer. I dette studiet kartla vi næringssøksområdene hos Antarktispetrell (Thalassoica antarctica) som hekker i verdens største koloni (Svarthammaren, Dronning Maud land) over en treårsperiode. Vi fant at det romlige overlappet mellom krillfiskerier og næringssøkende Antarktispetrell generelt var lite. Konkurranse mellom Antarktispetrell og krill-fiskerier er for tiden neglisjerbart, men kan øke hvis fiskeriet etter krill øker.

Ice cores provide temporal records of surface mass balance (SMB). Coastal areas of Antarctica have relatively high and variable SMB, but are under-represented in records spanning more than 100 years. Here we present SMB reconstruction from a 120 m-long ice core drilled in 2012 on the Derwael Ice Rise, coastal Dronning Maud Land, East Antarctica. Water stable isotope (δ18O and δD) stratigraphy is supplemented by discontinuous major ion profiles and continuous electrical conductivity measurements. The base of the ice core is dated to AD 1759 ± 16, providing a climate proxy for the past  ∼ 250 years. The core's annual layer thickness history is combined with its gravimetric density profile to reconstruct the site's SMB history, corrected for the influence of ice deformation. The mean SMB for the core's entire history is 0.47 ± 0.02 m water equivalent (w.e.) a−1. The time series of reconstructed annual SMB shows high variability, but a general increase beginning in the 20th century. This increase is particularly marked during the last 50 years (1962–2011), which yields mean SMB of 0.61 ± 0.01 m w.e. a−1. This trend is compared with other reported SMB data in Antarctica, generally showing a high spatial variability. Output of the fully coupled Community Earth System Model (CESM) suggests that, although atmospheric circulation is the main factor influencing SMB, variability in sea surface temperatures and sea ice cover in the precipitation source region also explain part of the variability in SMB. Local snow redistribution can also influence interannual variability but is unlikely to influence long-term trends significantly. This is the first record from a coastal ice core in East Antarctica to show an increase in SMB beginning in the early 20th century and particularly marked during the last 50 years.

Mass changes of polar ice sheets have an important societal impact, because they affect global sea level. Estimating the current mass budget of ice sheets is equivalent to determining the balance between surface mass gain through precipitation and outflow across the grounding line. For the Antarctic ice sheet, grounding line outflow is governed by oceanic processes and outlet glacier dynamics. In this study, we compute the mass budget of major outlet glaciers in the eastern Dronning Maud Land sector of the Antarctic ice sheet using the input/output method. Input is given by recent surface accumulation estimates (SMB) of the whole drainage basin. The outflow at the grounding line is determined from the radar data of a recent airborne survey and satellite-based velocities using a flow model of combined plug flow and simple shear. This approach is an improvement on previous studies, as the ice thickness is measured, rather than being estimated from hydrostatic equilibrium. In line with the general thickening of the ice sheet over this sector, we estimate the regional mass balance in this area at 3.15 ± 8.23 Gt a−1 according to the most recent SMB model results.

Ice rises situated in the ice-shelf belt around Antarctica have a spatially confined flow regime with local ice divides. Beneath the divides, ice stratigraphy often develops arches with amplitudes that record the divide's horizontal residence time and surface elevation changes. To investigate the evolution of Derwael Ice Rise, Dronning Maud Land, Antarctica, we combine radar and GPS data from three consecutive surveys, with a two-dimensional, full Stokes, thermomechanically coupled, transient ice-flow model. We find that the surface mass balance (SMB) is higher on the upwind and lower on the downwind slopes. Near the crest, the SMB is anomalously low and causes arches to form in the shallow stratigraphy, observable by radar. In deeper ice, arches are consequently imprinted by both SMB and ice rheology (Raymond effect). The data show how arch amplitudes decrease as along-ridge slope increases, emphasizing that the lateral positioning of radar cross sections is important for the arch interpretation. Using the model with three rheologies (isotropic with n=3,4.5 and anisotropic with n=3), we show that Derwael Ice Rise is close to steady state but is best explained using ice anisotropy and moderate thinning. Our preferred, albeit not unique, scenario suggests that the ice divide has existed for at least 5000 years and lowered at approximately 0.03 m a−1 over the last 3400 years. Independent of the specific thinning scenario, our modeling suggests that Derwael Ice Rise has exhibited a local flow regime at least since the Mid-Holocene.

The Alfred Wegener Institute, Helmholtz Centre for Polar and Marine Research (AWI) and the Federal Institute for Geosciences and Natural Resources (BGR) collected around 150 hours of new gravity, magnetic and ice-penetrating radar data from east and south of Princess Elisabeth station in Dronning Maud Land between 2013 and 2015. Survey lines were spaced 10 km apart. The 2013/2014 and 2014/2015 used different gravimeters; a LaCoste and Romberg AirSea gravimeter (LCR) at constant barometric altitude and a Gravimetric Technologies GT2A gravimeter at constant ground separation. Both surveys used a Scintrex Cs-3 caesium vapour magnetometer mounted in a tail boom with compensation for the airframe calculated using a fuselage-mounted three-component fluxgate magnetometer. The GT2A gravity data reflect the effects of short-wavelength density contrasts between basement rocks and the ice sheet more reliably than the LCR data. Cross-over analysis suggests the repeatability of data collection with the GT2A lies at the sub-milliGal level. A broad subglacial channel that separates eastern Sør Rondane from the Yamato Belgica Mountains is evident in the gravity data. In the south of the survey region, the data reveal a dendritic pattern of subglacial valleys that converge towards the SW. Strong NS-trending magnetic anomalies coincide with the Yamato-Belgica Mountains. Further west, subtler ESE-trending anomalies confirm proposals that the SE Dronning Maud Land province continues into the region south of eastern Sør Rondane. An unexpected feature of both data sets is the apparent termination of the anomaly patterns associated with the province at a NNW-trending anomaly running south of Princess Elisabeth.

We present implementations of vibroseis system configurations with a snowstreamer for over-ice long-distance seismic traverses (>100 km). The configurations have been evaluated in Antarctica on ice sheet and ice shelf areas in the period 2010–2014. We discuss results of two different vibroseis sources: Failing Y-1100 on skis with a peak force of 120 kN in the frequency range 10–110 Hz; IVI EnviroVibe with a nominal peak force of 66 kN in the nominal frequency range 10–300 Hz. All measurements used a well-established 60 channel 1.5 km snowstreamer for the recording. Employed forces during sweeps were limited to less than 80% of the peak force. Maximum sweep frequencies, with a typical duration of 10 s, were 100 and 250 Hz for the Failing and EnviroVibe, respectively. Three different concepts for source movement were employed: the Failing vibrator was mounted with wheels on skis and pulled by a Pistenbully snow tractor. The EnviroVibe was operated self-propelled on Mattracks on the Antarctic plateau. This lead to difficulties in soft snow. For later implementations the EnviroVibe with tracks was put on a polyethylene (PE) sled. The sled had a hole in the center to lower the vibrator baseplate directly onto the snow surface. With the latter setup, data production varied between 20 km/day for 6-fold and 40 km/day for single fold for 9 h/day of measurements. The combination of tracks with the PE-sled was especially advantageous on hard and rough surfaces because of the flexibility of each component and the relatively lose mounting. The systems presented here are suitable to obtain data of subglacial and sub-seabed sediment layers and englacial layering in comparable quality as obtained from marine geophysics and land-based explosive surveys. The large offset aperture of the streamer overcomes limitations of radar systems for imaging of steep along-track subglacial topography. With joint international scientific and logistic efforts, large-scale mapping of Antarctica's and Greenland's subglacial geology, ice-shelf cavity geometries and sea-bed strata, as well as englacial structures can be achieved.

The geology of East Antarctica and its correlation in major supercontinents is highly speculative, since only a very small part of it is exposed. Therefore a better connection between geology and geophysics is needed in order to correlate exposed regions with ice-covered, geophysically-defined, blocks. In Dronning Maud Land (DML), two distinct late Mesoproterozoic/early Neoproterozoic tectono-metamorphic provinces appear, separated by the major, NE-trending Forster Magnetic Anomaly and South Orvin Shear Zone. To the west of this lineament, the Maud Belt has clear affinities with Grenville-age continent-continent mobile belts. East of the Forster Magnetic Anomaly, juvenile rocks with early Neoproterozoic age (Rayner-age) and an accretionary character crop out. The international GEA-II expedition (2012) targeted a white spot on the geological map immediately to the E of the Forster Magnetic Anomaly. This area allows the characterization and ground-truthing of a large and mostly ice-covered region, the SE DML Province that had previously been interpreted as an older cratonic block. However, new SHRIMP/SIMS zircon analyses and their geochemistry indicates that the exposed basement consists of a ca. 1000-900 Ma juvenile terrane that is very similar to rocks in Sor Rondane. It lacks significant metamorphic overprint at the end of crust formation, but it shows medium to high-grade overprinting between ca. 630-520 Ma, associated with significant felsic melt production, including A-type granitoid magmatism. Therefore, the aeromagnetically distinct SE DML province does neither represent the foreland of a Late Neoproterozoic/EarlyPaleozoic mobile belt, nor a craton, as has previously been speculated. It more likely represents the more juvenile, westward continuation of Rayner-age crust (1000-900 Ma). To the west it abuts along the NE-trending Forster Magnetic Anomaly. The latter is interpreted as a suture, which separates typical Grenville-age crust of the Maud Belt (ca. 1200-1030 Ma) to the W from Rayner-age crust to the E. Therefore the larger eastern part of DML has clearly Indian affinities. Its juvenile character with a lack of metamorphic overprint at the end of crust formation points to an accretionary history along this part of the Indian segment of Rodinia, immediately following final Rodinia assembly.

This article highlights the field geology, geochronology and geochemistry of an important and previously unstudied region between eastern (Sør Rondane Mountains) and central Dronning Maud Land (DML). The area allows the characterisation and ground-truthing of a large and mostly ice-covered area that is geophysically distinct and which was previously interpreted as a potentially older cratonic block south of a Late Neoproterozoic/Early Paleozoic (LN/EP) mobile belt, as exposed in the Sør Rondane Mts. (SRM). SHRIMP/SIMS zircon analyses of 20 samples together with new geochemistry indicate that the exposed basement consists of a ca. 1000–900Ma juvenile terrane that is very similar to the juvenile rocks of the SW-Terrane of the SRM, a characteristic gabbro–trondhjemite–tonalite–granite (GTTG) suite, with normalised trace element patterns typical for subduction-related magmas and mostly positive initial epsilon Nd values. The area shows strong LN/EP crustal reworking, migmatisation and melt production, including 560–530Ma A-type magmatism. Therefore, this area is very similar to the SW-Terrane and differs only in the degree of LN/EP reworking. We interpret the SW-Terrane of Sør Rondane as a mega-boudin sandwiched in between rheologically weaker portions of similar oceanic arc terranes. Therefore, the study area, and thereby the aeromagnetically distinct SE DML province does neither represent the foreland of a LN/EP mobile belt, nor a craton, as speculated based on geophysical data alone. Instead, a large Tonian Oceanic Arc Super Terrane (TOAST) with significant extent emerges. Its western limit is represented by the Forster Magnetic Anomaly, which represents a suture to the Grenville-age Maud Belt. East of the TOAST, the Rayner Complex is similar in age but otherwise distinctly different. The Rayner Complex has a much longer history of island arc accretions with continent–continent collision at ca. 950Ma and it has markedly more evolved crust. In contrast, the TOAST has a pronounced juvenile character without significant inheritance and lacks metamorphic overprint immediately following crust formation. This indicates that it has not been an integral part of Rodinia. The eastern boundary of the TOAST is probably in the vicinity of the Yamato Mts., whilst its northern extension might be seen in the Vohibori Terrane (SW Madagascar), which in turn could correlate with the Arabian Nubian Shield. The LN/EP tectono-metamorphic overprint of the TOAST shows a slight decrease in ages from W to E, possibly indicating that it first amalgamated on its Kalahari side before it was attached to Rukerland/Indo-Antarctica.

The Kalahari Craton is an important building block of the supercontinent Rodinia, but its position with respect to other cratons is still controversially discussed. The Maud Belt in East Antarctica is part of the extensive Namaqua-Natal-Maud Orogen along which Kalahari collided with another continent during Rodinia assembly. One of the continents that have been suggested as collision partners for Kalahari is Western Australia, with the Pinjarra Orogen as the counterpart to the Maud Belt. We investigate this connection from a geochronological point of view. SHRIMP U/Pb zircon analyses of three metasedimentary samples from the Maud Belt date Grenville-age metamorphism within the orogen at ca. 1100–1060Ma. One sample was later affected by Pan-African metamorphism at ca. 540Ma. A second sample is interpreted as a molasse of the Maud Belt and was deposited in the Neoproterozoic. Detrital zircons from all three samples are consistent with derivation of the sediments predominantly from within the Namaqua-Natal-Maud Belt, with minor contributions from the Kalahari Craton. No clear Western Australian fingerprint could be detected in the detrital ages and a direct comparison between detrital zircon ages from the Maud Belt and the Northampton Complex (Pinjarra Orogen, Western Australia) showed distinct differences in the age spectra. Altogether, we consider a collision between Kalahari and south-western Laurentia a more likely scenario.

In this study, we analyze a large dataset of seismic signals, recorded by station TROLL in Dronning Maud Land, Antarctica. The signals, recorded in April–December 2012, came from sources near the edge of the ice shelves, at distances of 230–500 km from TROLL. The sources, which moved westward with time, could be associated with four large, tabular icebergs, drifting between 15° E and 8° W. Combining the seismological data with information from satellite remote sensing, we find that one-third of the signals can be attributed to individual icebergs. The trajectories of three of the associated icebergs are known through iceberg-tracking databases, whereas the fourth, a fragment of one of the other three, is untracked, and only scarce information is available from satellite imagery. The observed seismic signals exhibit a wide variety of frequency characteristics, from unstructured episodes to occurrences of iceberg harmonic tremor. Although we are not able to determine the exact cause of the signals, we classify them into five classes on a phenomenological basis. This study demonstrates the potential of regional seismic networks for iceberg monitoring as supplementary resources to information obtained with remote-sensing technologies.

Structural investigations in western Sør Rondane, eastern Dronning Maud Land (DML), provide new insights into the tectonic evolution of East Antarctica. One of the main structural features is the approximately 120 km long and several hundred meters wide WSW-ENE trending Main Shear Zone (MSZ). It is characterized by dextral high-strain ductile deformation under peak amphibolite-facies conditions. Crosscutting relationships with dated magmatic rocks bracket the activity of the MSZ between late Ediacaran to Cambrian times (circa 560 to 530 Ma). The MSZ separates Pan-African greenschist- to granulite-facies metamorphic rocks with “East African” affinities in the north from a Rayner-age early Neoproterozoic gabbro-tonalite-trondhjemite-granodiorite complex with “Indo-Antarctic” affinities in the south. It is interpreted to represent an important lithotectonic strike-slip boundary at a position close to the eastern margin of the East African-Antarctic Orogen (EAAO), which is assumed to be located farther south in the ice-covered region. Together with the possibly coeval left-lateral South Orvin Shear Zone in central DML, the MSZ may be related to NE directed lateral escape of the EAAO, whereas the Heimefront Shear Zone and South Kirwanveggen Shear Zone of western DML are part of the south directed branch of this bilateral system.

The geology of Sør Rondane has been the focus of intense research and occupies a key position for reconstructing the late Neoproterozoic to early Paleozoic geodynamic evolution in eastern Dronning Maud Land (DML). Sør Rondane appears to be located close to the supposed intersection of the East African-Antarctic Orogen (EAAO) and the Kuunga Orogen. The western part of Sør Rondane is subdivided in two distinct terranes. The amphibolite to granulite-facies NE terrane is mainly composed of metasupracrustal rocks, with detrital zircon ages in part younger than 750 Ma, deposited on older basement of unknown, possibly Rayner-type, crust (Shiraishi et al., 2008). Metamorphism has been dated by U-Pb on zircon at ca. 640-600 Ma and amphibolite-facies retrogression dated at ca. 590-530 Ma. The SW terrane is subdivided by the Main Shear Zone (MSZ) into two lithothectonic units, i.e. Pan- African greenschist- to granulite-facies metamorphic rocks with “East African” affinities in the N and a Rayner-age early Neoproterozoic gabbro-tonalite-trondhjemite-granodiorite (GTTG) complex with “Indo-Antarctic” affinities in the S. The GTTG complex has suffered Pan-African greenschist- to lower amphibolite-facies thermal overprint, but also contains large domains with only weak deformation except for its northern margin close to the MSZ. The deformation there is related to high shear strain along this structure. New zircon crystallisation ages of the GTTG cluster around 1000-930 Ma. It is interpreted to have formed along a juvenile oceanic arc, in which the wide age range might indicate a long-lasting accretionary orogen. The MSZ is characterized by a right-lateral sense of movement and high-strain ductile deformation under peak amphibolite-facies conditions. The structure can be traced over a distance of ca. 120 km between Lågkollane in the W and Lunckeryggen in the E and reaches several hundred meters in width. The MSZ cannot be traced further to the W where it seems to terminate at the north-eastern border of the NW-SE oriented prominent magnetically defined SE DML Province. The north-eastern border zone may coincide with a significant dextral shear zone that runs from the Schirmacher Oasis into the region S of Sør Rondane (Schirmacher- Rondane Lineament). The SE DML Province most likely consists of Rayner-age (1000-900 Ma) crust with evidence of intense Pan-African reworking indicated by new geochronological data and was part of a large Tonian Oceanic Arc Super Terrane (TOAST). The continuation of the MSZ into eastern Sør Rondane and beyond is not clear either, since it appears to terminate at a N-S oriented region with low magnetic signatures (central Sør Rondane corridor) that is possibly related to extensional tectonics. Crosscutting relationships with dated magmatic rocks bracket the activity of the MSZ between Latest Ediacaran to Cambrian times (c. 560- 530 Ma). Based on new combined aeromagnetic and structural results from a four-seasons survey of the greater Sør Rondane region, we propose that the crustal structural architecture of eastern DML and is strongly influenced by N-directed (with Africa/Antarctica restored to its original position in Gondwana) lateral extrusion of the EAAO. This process was likely driven by the combination of (i) indentation of the SE DML block towards the conjugate stable Kalahari- Grunehogna cratonic foreland, (ii) extensional collapse of the previously (c. 580-550 Ma) thickened and gravitational instable crust of central DML, and (iii) large-scale tectonic escape of crustal blocks in eastern DML along major shear zones such as the Schirmacher Rondane Lineament and MSZ towards an unconstrained yet unknown region at a lateral position of the EAAO.

The paleo-topography of East Antarctica is highly relevant for the development of the East Antarctic ice-sheet. This ice-sheet originated probably as small ice caps and in the elevated areas of the cratons in East Antarctica around the Eocene/Oligocene boundary. East Antarctica contains three mountain ranges: the latitudinal Dronning Maud Land Mountains (DML), the longitudinal Transantarctic Mountains (TAM) and the sub-glacial Gamburtsev Mountains (GM). The 1500 km long, coast-parallel Dronning Maud Land Mountains probably resulted in a significant amount of precipitation prior to the initiation of the 34 Ma glaciation history of East Antarctica. Thus, the paleo-topography should be used as an important input parameter for the glaciation history.

Migratory routes and the areas used during winter have probably been selected to maximize fitness by providing favorable environmental conditions outside the breeding season. In polar environments, because of the extreme winter weather, most breeding species migrate to encounter better conditions in areas that can differ between and also within species. Using geolocation sensors, we found that south polar skuas Catharacta maccormicki from 2 distant populations breeding on the Antarctic continent along the Atlantic and Indian Oceans migrate northward to winter in tropical Indian Ocean and in temperate North Pacific waters, respectively. Most individuals from each population winter in different environmental conditions, with water temperatures ranging from 16 to 29°C. Nevertheless, they have very similar activity patterns, spending more than 80% of their time on the water, and their feather δ15N values suggest that they probably feed at similar trophic levels during the molt. During overwintering, the overall and constant low activity level may be partly imposed by molting constraints, but it also suggests that trophic conditions are good for skuas. The wintering areas of the species correspond to sectors of high concentrations of breeding or wintering tropical, Northern, and Southern Hemisphere seabird species that are likely to be kleptoparasitized by skuas. A certain degree of individual variation exists within each population, which induces a spatial overlap in the wintering grounds of distant breeding populations. These results have potential important consequences in terms of fitness, genetic divergence, and susceptibility to climate change and marine pollution. KEYWORDS: Catharacta maccormicki · Geolocators · Migration · Population-specific strategies · Stable isotopes.

We present results of a multi-methodological approach to characterize the flow regime of West Ragnhild Glacier, the widest glacier in Dronning Maud Land, Antarctica. A new airborne radar survey points to substantially thicker ice (>2000 m) than previously thought. With a discharge estimate of 13–14 Gt yr−1, West Ragnhild Glacier thus becomes of the three major outlet glaciers in Dronning Maud Land. Its bed topography is distinct between the upstream and downstream section: in the downstream section (<65 km upstream of the grounding line), the glacier overlies a wide and flat basin well below the sea level, while the upstream region is more mountainous. Spectral analysis of the bed topography also reveals this clear contrast and suggests that the downstream area is sediment covered. Furthermore, bed-returned power varies by 30 dB within 20 km near the bed flatness transition, suggesting that the water content at bed/ice interface increases over a short distance downstream, hence pointing to water-rich sediment. Ice flow speed observed in the downstream part of the glacier (~250 m yr−1) can only be explained through very low basal friction, leading to a substantial amount of basal sliding in the downstream 65 km of the glacier. All the above lines of evidence (sediment bed, wetness and basal motion) and the relatively flat grounding zone give the potential for West Ragnhild Glacier to be more sensitive to external forcing compared to other major outlet glaciers in this region, which are more stable due to their bed geometry (e.g. Shirase Glacier).

This article investigates the annual cycle observed in the Antarctic baseline aerosol scattering coefficient, total particle number concentration, and particle number size distribution (PNSD), as measured at Troll Atmospheric Observatory. Mie theory shows that the annual cycles in microphysical and optical aerosol properties have a common cause. By comparison with observations at other Antarctic stations, it is shown that the annual cycle is not a local phenomenon, but common to central Antarctic baseline air masses. Observations of ground-level ozone at Troll as well as backward plume calculations for the air masses arriving at Troll demonstrate that the baseline air masses originate from the free troposphere and lower stratosphere region, and descend over the central Antarctic continent. The Antarctic summer PNSD is dominated by particles with diameters <100 nm recently formed from the gas-phase despite the absence of external sources of condensible gases. The total particle volume in Antarctic baseline aerosol is linearly correlated with the integral insolation the aerosol received on its transport pathway, and the photooxidative production of particle volume is mostly limited by photooxidative capacity, not availability of aerosol precursor gases. The photooxidative particle volume formation rate in central Antarctic baseline air is quantified to 207 ±4 μm3/(MJ m). Further research is proposed to investigate the applicability of this number to other atmospheric reservoirs, and to use the observed annual cycle in Antarctic baseline aerosol properties as a benchmark for the representation of natural atmospheric aerosol processes in climate models.