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Nearly three decades of stable isotope ratios and surface mass balance (SMB) data from eight shallow firn cores retrieved at Fimbul Ice Shelf, East Antarctica, in the Austral summers 2009–2011 have been investigated. An additional longer core drilled in 2000/2001 extends the series back to the early eighteenth century. Isotope ratios and SMB from the stacked record of all cores were also related to instrumental temperature data from Neumayer Station on Ekström Ice Shelf. Since the second half of the twentieth century, the SMB shows a statistically significant negative trend, whereas the δ18O of the cores shows a significant positive trend. No trend is found in air temperature at the nearest suitable weather station, Neumayer (available since 1981). This does not correspond to the statistically significant positive trend in Southern Annular Mode (SAM) index, which is usually associated with a cooling of East Antarctica. SAM index and SMB are negatively correlated, which might be explained by a decrease in meridional exchange of energy and moisture leading to lower precipitation amounts. Future monitoring of climate change on the sensitive Antarctic ice shelves is necessary to assess its consequences for sea level change.

The effects of nunataks on temperature profiles and wind patterns are studied using simulations from the Weather Research and Forecasting model. Simulations are compared to hourly observations from an automatic weather station located at the Troll Research Station in Dronning Maud Land. Areas of bare ground have been implemented in the model, and the simulations correspond well with meteorological measurements acquired during the 4 day simulation period. The nunataks are radiatively heated during daytime, and free convection occurs in the overlying atmospheric boundary layer. The inflow below the updraft forces strong horizontal convergence at the surface, whereas weaker divergence appears aloft. In a control run with a completely ice-covered surface, the convection is absent. In situ observations carried out by a remotely controlled balloon and a small model airplane compare well with model temperature profiles, but these are only available over the ice field upwind to the nunatak.

Atmospheric aerosol samples were collected over the Southern Ocean (SO) and coastal East Antarctica (CEA) during the austral summer of 2010/11. Samples were analysed for trace elements, including Na, Mg, K, Al, Fe, Mn, Ni, Cd and Se, by inductively coupled plasma mass spectrometry (ICP-MS). The mean atmospheric concentrations over the SO were 1100 ng m−3 for Na, 190 ng m−3 for Mg, 150 ng m−3 for Al, 14 ng m−3 for Fe, 0.46 ng m−3 for Mn and 0.25 ng m−3 for Se. Over CEA, the mean concentrations were 990 ng m−3 for Na, 180 ng m−3 for Mg, 190 ng m−3 for Al, 26 ng m−3 for Fe, 0.70 ng m−3 for Mn and 0.29 ng m−3 for Se. Particle size distributions, enrichment factors (EFs) and correlation analysis indicate that Na, Mg and K mainly came from the marine source, while Al, Fe and Mn were mainly from the crustal source, which also contributed to Mg and K over CEA. High EFs were associated with Ni, Cd and Se, suggesting likely contributions from mixed sources from the Antarctic continent, long-range transport, marine biogenic emissions and anthropogenic emissions. Sea-salt elements (Na, Mg, K) were mainly accumulated in the coarse mode, and crustal elements (Al, Fe, Mn) presented a bimodal size distribution pattern. Bioactive elements (Fe, Ni, Cd) were enriched in the fine mode, especially with samples collected over the SO, possibly affecting biogeochemical cycles in this oceanic region. Keywords: Southern Ocean; coastal East Antarctica; trace elements; size distribution; sources.

Enhancement of ocean alkalinity using calcium compounds, e.g., lime has been proposed to mitigate further increase of atmospheric CO2 and ocean acidification due to anthropogenic CO2 emissions. Using a global model, we show that such alkalinization has the potential to preserve pH and the saturation state of carbonate minerals at close to today's values. Effects of alkalinization persist after termination: Atmospheric CO2 and pH do not return to unmitigated levels. Only scenarios in which large amounts of alkalinity (i.e., in a ratio of 2:1 with respect to emitted CO2) are added over large ocean areas can boost oceanic CO2 uptake sufficiently to avoid further ocean acidification on the global scale, thereby elevating some key biogeochemical parameters, e.g., pH significantly above preindustrial levels. Smaller-scale alkalinization could counteract ocean acidification on a subregional or even local scale, e.g., in upwelling systems. The decrease of atmospheric CO2 would then be a small side effect.

We report ground-based measurements of the polar middle atmosphere made using a 230–250 GHz passive microwave radiometer deployed at Troll station (72°01′S 02°32′E, L shell of L = 4.8), Antarctica. Our observations show enhanced mesospheric nitric oxide (NO) volume mixing ratio (VMR) during a series of small recurrent geomagnetic storms in the 2008 austral winter, reaching 1.2 ppmv on day 200 (18 July). The Lomb normalized periodogram of the NO VMR time series averaged over 65-80 km for days 130 to 220 of 2008 (9 May to 7 August) shows a peak exceeding the 95% confidence limit at 25.8 days, close to the synodic rotation period for low-latitude solar coronal holes. The highest correlations between the radiometer NO VMR data and trapped and quasi-trapped electron count rates for L = 3.5-5.5 from the Polar Orbiting Environment Satellites 90° telescope are for the >30 keV (90e1) channel (rmax = 0.56, lag time of 5.1 days) and >100 keV (90e2) channel (rmax = 0.57, lag time of 4.4 days). Maximum correlation between NO VMR and the >700 keV (90P6) channel data is lower but lag times are close to zero. Superposed epoch analyses for the eight most significant geomagnetic storm periods and three Carrington rotations (2070-2072) within the 90 day observation period indicate that significant NO abundance observed at 65-80 km in the Antarctic mesosphere may be produced directly by >200 keV electron precipitation or originate from a source at higher altitudes, e.g., production by >30 keV electrons followed by downward transport.

In this study, we present evidence that Antarctic and Arctic sea ice act as sink for atmospheric CO2 during periods of snowmelt and surface flooding. The CO2 flux measured directly at the flooded sea ice surface (Fflood) constituted a net CO2 sink of −1.1 ± 0.9 mmol C m−2 d−1 (mean ± 1 SD), which was an order of magnitude higher than the flux measured at the snow-air surface (Fsnow) and bare ice surface (Fice). The Fsnow/Fflood ratio decreased with increasing water equivalent of snow and superimposed-ice, suggesting that the properties of snow and superimposed-ice formation affect the magnitude of the CO2 flux. The Fsnow/Fflood ratio ranged from 0.1 to 0.5, illustrating that 50–90% of the potential flux at the flooded surface was reduced due to the presence of snow/superimposed-ice. Hence, snow cover properties and superimposed-ice play an important role in the CO2 fluxes across the sea ice-snow-atmosphere interface.

As part of the 2009 Operation Ice Bridge campaign, the NASA DC-8 aircraft was used to fill the data-time gap in laser observation of the changes in ice sheets, glaciers and sea ice between ICESat-I (Ice, Cloud, and land Elevation Satellite) and ICESat-II. Complementing the cryospheric instrument payload were four in situ atmospheric sampling instruments integrated onboard to measure trace gas concentrations of CO2, CO, N2O, CH4, water vapor and various VOCs (Volatile Organic Compounds). This paper examines two plumes encountered at high altitude (12 km) during the campaign; one during a southbound transit flight (13°S) and the other at 86°S over Antarctica. The data presented are especially significant as the Southern Hemisphere is heavily under-sampled during the austral spring, with few if any high-resolution airborne observations of atmospheric gases made over Antarctica. Strong enhancements of CO, CH4, N2O, CHCl3, OCS, C2H6, C2H2 and C3H8 were observed in the two intercepted air masses that exhibited variations in VOC composition suggesting different sources. The transport model FLEXPART showed that the 13°S plume contained predominately biomass burning emissions originating from Southeast Asia and South Africa, while both anthropogenic and biomass burning emissions were observed at 86°S with South America and South Africa as indicated source regions. The data presented here show evidence that boundary layer pollution is transported from lower latitudes toward the upper troposphere above the South Pole, which may not have been observed in the past.

We compare the present and last interglacial periods as recorded in Antarctic water stable isotope records now available at various temporal resolutions from six East Antarctic ice cores: Vostok, Taylor Dome, EPICA Dome C (EDC), EPICA Dronning Maud Land (EDML), Dome Fuji and the recent TALDICE ice core from Talos Dome. We first review the different modern site characteristics in terms of ice flow, meteorological conditions, precipitation intermittency and moisture origin, as depicted by meteorological data, atmospheric reanalyses and Lagrangian moisture source diagnostics. These different factors can indeed alter the relationships between temperature and water stable isotopes. Using five records with sufficient resolution on the EDC3 age scale, common features are quantified through principal component analyses. Consistent with instrumental records and atmospheric model results, the ice core data depict rather coherent and homogenous patterns in East Antarctica during the last two interglacials. Across the East Antarctic plateau, regional differences, with respect to the common East Antarctic signal, appear to have similar patterns during the current and last interglacials. We identify two abrupt shifts in isotopic records during the glacial inception at TALDICE and EDML, likely caused by regional sea ice expansion. These regional differences are discussed in terms of moisture origin and in terms of past changes in local elevation histories, which are compared to ice sheet model results. Our results suggest that elevation changes may contribute significantly to inter-site differences. These elevation changes may be underestimated by current ice sheet models.

We report the first ground-based passive microwave observations made from Troll station, Antarctica, which show enhanced mesospheric nitric oxide (NO) volume mixing ratio reaching levels of 1.2 ppmv, or 2–3 orders of magnitude above background, at 70–80 km during small, relatively isolated geomagnetic storms in 2008. The mesospheric NO peaked 2 days after enhanced NO at higher altitudes (110–150 km) measured by the SABER satellite, and 2 days after peaks in the >30 keV and >300 keV electron flux measured by POES, although the 300 keV electron flux remained high. High time resolution data shows that mesospheric NO was enhanced at night and decayed during the day and built up to high levels over a period of 3–4 days. The altitude profile of mesospheric NO suggests direct production by ∼300 keV electron precipitation. Simulations using the Sodankylä Ion and Neutral Chemistry model show that the delay between thermospheric and mesospheric NO enhancements was primarily a result of the weaker production rate at lower altitudes by ∼300 keV electrons competing against strong day-time losses.

We use observations of N2O and mean age to identify realistic transport in models in order to explain their ozone predictions. The results are applied to 15 chemistry climate models (CCMs) participating in the 2010 World Meteorological Organization ozone assessment. Comparison of the observed and simulated N2O, mean age and their compact correlation identifies models with fast or slow circulations and reveals details of model ascent and tropical isolation. This process-oriented diagnostic is more useful than mean age alone because it identifies models with compensating transport deficiencies that produce fortuitous agreement with mean age. The diagnosed model transport behavior is related to a model's ability to produce realistic lower stratosphere (LS) O3 profiles. Models with the greatest tropical transport problems compare poorly with O3 observations. Models with the most realistic LS transport agree more closely with LS observations and each other. We incorporate the results of the chemistry evaluations in the Stratospheric Processes and their Role in Climate (SPARC) CCMVal Report to explain the range of CCM predictions for the return-to-1980 dates for global (60°S–60°N) and Antarctic column ozone. Antarctic O3 return dates are generally correlated with vortex Cly levels, and vortex Cly is generally correlated with the model's circulation, although model Cl chemistry and conservation problems also have a significant effect on return date. In both regions, models with good LS transport and chemistry produce a smaller range of predictions for the return-to-1980 ozone values. This study suggests that the current range of predicted return dates is unnecessarily broad due to identifiable model deficiencies.

The horizontal wind data from the standard version of Canadian Middle Atmosphere Model Data Assimilation System (CMAM-DAS) for the years 2006–2008 are analyzed to obtain the global structure and seasonal variability of the semidiurnal tide (SDT) in the mesosphere. The modeled amplitudes and phases of the SDTs at single stations from middle/high northern latitudes are quite similar to those observed by radars. The primary nonmigrating tides identified in both the meridional wind and zonal wind semidiurnal spectra at 88 km include the westward propagating wave numbers s = 1 (SW1), 3 (SW3), 4 (SW4), 6 (SW6), the standing s = 0 (S0), and the eastward propagating s = 2 (SE2). The migrating SDT (SW2) amplitude maxima usually occur at 40°N–60°N during December–February and August–September, and also at 40°S–60°S in April–May, with the dominance of (2, 4) during October–April and (2, 3) and (2, 5) dominance for other months. The CMAM-DAS is quite successful in reproducing the dominance of SW1 in the Antarctic summer mesosphere. The modeled SW1 shows very good overall agreement in both amplitude and phase with wind measurements from UARS High Resolution Doppler Imager and Wind Imaging Interferometer (UARS-HRDI/WINDII) and from TIMED Doppler Interferometer (TIDI). The CMAM-DAS analyses for SW3, SW4, SW6, and S0 are also in reasonable agreement with those determined from the HRDI/WINDII or TIDI wind measurements. This work provides further evidence for the tidal forcing from below.

The latent heat fluxes (LHF) and sensible heat fluxes (SHF) over the Southern Ocean from six different data sets are inter-compared for the period 1988- 2000. The six data sets include three satellite-based products, namely, the second version of the Goddard Satellite-Based Surface Turbulent Fluxes data set (GSSTF-2), the third version of the Hamburg Ocean Atmosphere Parameters and Fluxes from Satellite Data (HOAPS-3) and the Japanese Ocean Fluxes Data Sets with Use of Remote Sensing Observations (J-OFURO); two global reanalysis products, namely, the National Centers for Environmental Prediction-Department of Energy Reanalysis 2 data set (NCEP-2) and the European Centre for Medium-Range Weather Forecasts 40 Year Re-analysis data set (ERA-40); and the Objectively Analyzed Air-Sea Fluxes for the Global Oceans data set (OAFlux). All these products reveal a similar pattern in the averaged flux fields. The zonal mean LHF fields all exhibit a continuous increase equatorward. With an exception of HOAPS-3, the zonal mean SHF fields display a minimum value near 50°S, increasing both pole- and equatorward. The differences in the standard deviation for LHF are larger among the six data products than the differences for SHF. Over the regions where the surface fluxes are significantly influenced by the Antarctic Oscillation and the Pacific-South American teleconnection, the values and distributions of both LHF and SHF are consistent among the six products. It was found that the spatial patterns of the standard deviations and trends of LHF and SHF can be explained primarily by sea-air specific humidity and temperature differences; wind speed plays a minor role. Keywords: Latent heat flux; sensible heat flux; Southern Ocean.

Clouds and the Earth's radiant energy system (CERES) is a satellite-based remote sensing system designed to monitor the Earth's radiation budget. In this paper we examine uncertainties in the angular distribution models (ADMs) used by CERES over permanently snow covered surfaces with clear skies. These ADMs are a key part of the CERES data processing algorithms, used to convert the observed upwelling radiance to an estimate of the upwelling hemispheric flux. We model top-of-atmosphere anisotropic reflectance factors using an atmospheric radiative transfer model with a lower boundary condition based on extensive reflectance observations made at Dome C, Antarctica. The model results and subsequent analysis show that the CERES operational clear-sky permanent-snow ADMs are appropriate for use over Dome C, with differences of less than 5% between the model results and the ADMs at most geometries used by CERES operationally. We show that the uncertainty introduced into the flux estimates through the use of the modeled radiances used in the ADM development is small when the fluxes are averaged over time and space. Finally, we show that variations in the angular distribution of radiance at the top of the atmosphere due to atmospheric variability over permanently snow covered regions are in most cases unlikely to mask the real variations in flux caused by these atmospheric variations.

Spectral albedo and bidirectional reflectance of snow were measured at Dome C on the East Antarctic Plateau for wavelengths of 350–2400 nm and solar zenith angles of 52°–87°. A parameterization of bidirectional reflectance, based on those measurements, is used as the lower boundary condition in the atmospheric radiation model SBDART to calculate radiance and flux at the top of the atmosphere (TOA). The model's atmospheric profile is based on radiosoundings at Dome C and ozonesoundings at the South Pole. Computed TOA radiances are integrated over wavelength for comparison with the Clouds and the Earth's Radiant Energy System (CERES) shortwave channel. CERES radiance observations and flux estimates from four clear days in January 2004 and January 2005 from within 200 km of Dome C are compared with the TOA radiances and fluxes computed for the same solar zenith angle and viewing geometry, providing 11,000 comparisons. The measured radiance and flux are lower than the computed values. The median difference is about 7% for CERES on Terra, and 9% on Aqua. Sources of uncertainty in the model and observations are examined in detail and suggest that the measured values should be less than the computed values, but only by 1.7% ± 4%. The source of the discrepancy of about 6% cannot be identified here; however, the modeled values do agree with observations from another satellite instrument (Multiangle Imaging Spectroradiometer), suggesting that the CERES calibration must be considered a possible source of the discrepancy.

Sensitivity studies with global climate models show that, by their influence on the radiation balance, Antarctic clouds play a major role in the climate system, both directly at high southern latitudes and indirectly globally, as the local circulation changes lead to global teleconnections. Unfortunately, observations of cloud distribution in the Antarctic are limited and often of low quality because of the practical difficulty in observing clouds in the harsh Antarctic environment. The best surface observations suggest that the fractional cloud cover at the South Pole is around 50–60% in all seasons, whereas the cloud cover rises to around 80–90% close to the coast of the continent. Microphysical observations of cloud parameters are also very sparse in the Antarctic. However, the few measurements that do exist show predominantly ice-crystal clouds across the interior, with mixed-phase clouds close to the coasts. Crystal sizes vary from 5 to 30 mm (effective radius) in the interior to somewhat larger ice crystals and water drops near the coast. A wide range of crystal shapes is observed at all sites. This review considers the available cloud observations and highlights the importance of Antarctic clouds and the need for better observations in the future.

Observations of three bands of westward flow and two countercurrents, spanning roughly 50 km from the ice-shelf edge in front of the Fimbul Ice Shelf (prime meridian) in Antarctica, are presented. A comparison with a numerical model and the proximity of two of these current cores to the ice shelf suggest that they split from the Antarctic Coastal Current because of the influence of sea ice on the surface drag. A comparison with previous studies suggests that the other core is the current associated with the Antarctic Slope Front. Because the Fimbul ice shelf overhangs the continental shelf, the Antarctic Coastal Current displaces offshore, getting close to the Antarctic Slope Front. The obtained structure is derived from conductivity–temperature–depth geostrophic velocities from February 2005, referenced with detided acoustic Doppler current profiler velocities.

An extreme precipitation event that influenced almost the whole polar plateau of Dronning Maud Land, Antarctica, is investigated using Antarctic Mesoscale Prediction System archive data. For the first time a high-resolution atmospheric model especially adapted for polar regions was used for such a study in Dronning Maud Land. The outstanding event of 21–25 February 2003 was connected to a strong north-westerly flow, caused by a blocking high above eastern Dronning Maud Land, that persisted for several days and brought unusually large levels of moisture to the Antarctic Plateau. This weather situation is most effective in bringing precipitation to high-altitude interior Antarctic ice-core drilling sites, where precipitation in the form of diamond dust usually dominates. However, a few such precipitation events per year can account for a large percentage of the annual accumulation, which can cause a strong bias in ice-core data. Additionally, increased temperatures and wind speeds during these events need to be taken into account for the correct climatic interpretation of ice cores. A better understanding of the frequency of occurrence of intermittent precipitation in the interior of Antarctica in past and future climates is necessary for both palaeoclimatological studies and estimates of future sea-level change.

The atmospheric observatory at the Norwegian Research Station Troll in Queen Maud Land, Antarctica, holds, since February 2007, the first all-year Antarctic atmospheric aerosol particle number size distribution measurements. These are colocated with measurements of the aerosol absorption and spectral scattering coefficients. In June 2007, this instrument set observed an aerosol whose properties were indicative of a biomass burning aerosol. These properties included two log-normal size distribution modes with median particle diameters of 0.105 μm and 0.36 μm, sharply falling off to smaller and larger sizes, and peaks in scattering and absorption coefficient. With backward plume calculations of the Lagrangian transport model FLEXPART and the MODIS fire activity product, a source-receptor relationship was established between biomass burning events in Central Brazil and the aerosol seen at Troll. This is the first direct evidence that the Antarctic continent is susceptible to emissions from as far north as Southern tropical latitudes.

The Troll Atmospheric Station in Antarctica (72°01?S, 2°32?E, 1309 m a.s.l.) was established and put into operation in early 2007. The main foci of the measurement programme are pollution and aerosols in the transition zone between the coastal zone and the inland ice plateau, complementing existing observation programmes along the Antarctic coast and on the Antarctic Plateau. After one year of operation, the monitoring programme is fully operative, and a comprehensive set of data is being analysed. As far as comparable data are available, there is satisfactory agreement between previous and new data. Both aerosol data and measurements of pollution indicate the episodic influence of coastal air masses throughout the year. Background values of medium long-lived pollutants such as CO, O3 and Hg are up to 50% lower than at corresponding Arctic sites (depending on the season), but are still significant. Total ozone and UV doses manifest the recurring Antarctic stratospheric ozone hole, which was moderately severe, but very persistent in 2007. Specific episodes of elevated aerosol concentration and mercury activation are currently under detailed investigation, and will be published separately.

Observations of snow properties, superimposed ice, and atmospheric heat fluxes have been performed on first-year and second-year sea ice in the western Weddell Sea, Antarctica. Snow in this region is particular as it does usually survive summer ablation. Measurements were performed during Ice Station Polarstern (ISPOL), a 5-week drift station of the German icebreaker RV Polarstern. Net heat flux to the snowpack was 8 W m−2, causing only 0.1 to 0.2 m of thinning of both snow cover types, thinner first-year and thicker second-year snow. Snow thinning was dominated by compaction and evaporation, whereas melt was of minor importance and occurred only internally at or close to the surface. Characteristic differences between snow on first-year and second-year ice were found in snow thickness, temperature, and stratigraphy. Snow on second-year ice was thicker, colder, denser, and more layered than on first-year ice. Metamorphism and ablation, and thus mass balance, were similar between both regimes, because they depend more on surface heat fluxes and less on underground properties. Ice freeboard was mostly negative, but flooding occurred mainly on first-year ice. Snow and ice interface temperature did not reach the melting point during the observation period. Nevertheless, formation of discontinuous superimposed ice was observed. Color tracer experiments suggest considerable meltwater percolation within the snow, despite below-melting temperatures of lower layers. Strong meridional gradients of snow and sea-ice properties were found in this region. They suggest similar gradients in atmospheric and oceanographic conditions and implicate their importance for melt processes and the location of the summer ice edge.